Francis MatthewsCaptain Scarlet (voice)
Ed BishopCaptain Blue (voice)
Donald GrayColonel White / Captain Black / The Mysterons (voice)
Cy GrantLieutenant Green (voice)
Elizabeth MorganDestiny Angel / Rhapsody Angel / Harmony Angel (voice)
Gary FilesCaptain Magenta (voice)
David Healy(voice) (credit only)
Charles TingwellLieutenant Dean / Captain Brown / Agent 042 / Various Characters (voice)
